Study of electric field distribution on plasma and plasma catalysis reactor for different electrode configurations and pellet sizes

Authors

  • J. V. Deo School of Electrical Sciences, Indian Institute of Technology Goa
  • A. Madhukar School of Electrical Sciences, Indian Institute of Technology Goa

DOI:

https://doi.org/10.14311/ppt.2024.3.54

Keywords:

plasma catalysis, COMSOL multiphysics 6.0, diesel engine exhaust treatmnet, pellet size, electrode configuration, Non thermal plasma, optimal diameter

Abstract

In various non thermal plasma based applications, the dynamics of electric fields and charged particle interactions are crucial. In order to find an efficient plasma reactor, the effects of different electrode configurations for the plasma approach and pellet packaging & optimal sizing for the plasma catalysis approach were studied for 6 different types of volume discharge and surface discharge reactor using COMSOL Multiphysics 6.0. The different electrode configurations viz. concentric cylindrical, square and helical as volume discharged reactors and floating & 2 types of non-floating electrodes as surface discharge reactors are considered. The effect of different size (diameter 1/3/5 mm) of pellets were studied for helical and cylindrical plasma reactors for plasma catalysis. The simulated results were then experimentally verified and validated for production of ozone and the conversion or reduction of NOx from diesel exhaust.

References

M. Mortazavi, L. Amato, N. Manivannan, and W. Balachandran. Modelling of electric field distribution in a non-thermal plasma reactor using comsol multiphysics®, 2020. URL: https://www.comsol.com/paper/modelling-of-electric-field-distribution-in-a-non-thermal-plasma-reactor-using-comsol-multiphysics-95241.

A. Madhukar and B. Rajanikanth. Cascaded plasma–ozone injection system: A novel approach for controlling total hydrocarbon emission in diesel exhaust. Plasma Chemistry and Plasma Processing, 39:845–862, 2019. doi:10.1007/s11090-019-09959-8.

B. Chun, H. Lee, C. Nam, et al. Plasma/catalyst system for reduction of NOx in diesel engine exhaust. SAE Technical Paper 2000-01-2897, pages 2744–2748, 2000. doi:10.4271/2000-01-2897.

B. Penetrante, M. Hsiao, B. Merritt, et al. Comparison of electrical discharge techniques for nonthermal plasma processing of NO in N/sub 2/. IEEE Transactions on Plasma Science, 23(4):679–687, 1995. doi:10.1109/27.467990.

M. Chen, K. Takashima, and A. Mizuno. Effect of pellet-diameter on discharge characteristics and performance of a packed bed reactor. Int. J. Plasma Environ. Sci. Technol, 7(1):89–95, 2013. doi:10.34343/ijpest.2013.07.01.089.

S. Bhattacherjee and S. Mohapatro. Spike electrode-based DBD reactor for improved electric discharge power toward better diesel engine exhaust treatment at low applied voltage. IEEE Transactions on Plasma Science, 52(1):58–66, 2023. doi:10.1109/TPS.2023.3342028.

K. Takaki, M. Shimizu, S. Mukaigawa, and T. Fujiwara. Effect of electrode shape in dielectric barrier discharge plasma reactor for NOx removal. IEEE Transactions on Plasma Science, 32(1):32–38, 2004. doi:10.1109/TPS.2004.823973.

T. Hammer, T. Kappes, and M. Baldauf. Plasma catalytic hybrid processes: gas discharge initiation and plasma activation of catalytic processes. Catalysis today, 89(1–2):5–14, 2004. doi:10.1016/j.cattod.2003.11.001.

H. Wedaa, M. Abdel-Salam, A. Ahmed, and A. Mizuno. NO removal using dielectric barrier discharges in a multirod reactor stressed by AC and pulsed high voltages. IEEE Transactions on Dielectrics and Electrical Insulation, 18(5):1743–1751, 2011. doi:10.1109/TDEI.2011.6032846.

S. Vijay, A. Madhukar, and B. Rajanikanth. Catalyzing diesel exhaust through discharge plasma in a reactor packed with lignite ash/waste ceramic tiles: role of pellet diameter on DeNOx efficiency. In International Conference on Pollution Control for Clean Environment (ICPCCE-2023), 2023.

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Published

2024-12-03

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